Decolourization of Disperse Blue 3 Dye by Electro Coagulation Process Using Al and Fe Electrodes –Application of the Artificial Neural Network Model

Document Type : Research Article

Authors

1 University of Sciences and Technology, Faculty of Mechanical and Process Engineering/Environmental Department, BP 32, El-Alia 16111, Algiers, ALGERIA

2 Laboratory of Storage and Valorisation of Renewable Energies, Faculty of Chemistry, (USTHB), BP 32, 16111, Algiers, ALGERIA

Abstract

Contamination in wastewater is a major issue in the present world, Disperse blue 3 dye (DB3) removal was studied by an electrocoagulation process using Al and Fe electrodes. The experiments were performed with synthetic solutions in batch mode. The effect of the operating parameters like the electrolysis time, current density, initial pH, conductivity, inter-electrode distance, and initial dye concentration, has been investigated. The results show high discoloration efficiency, reaching 98 and 96% with Al and Fe electrodes respectively. The optimum condition of the EC process was electrolysis times of 70 and 30 min, current densities of 139 and 93 mA/cm², initial pH 5, the conductivity of 5.67 mS/cm, and inter-electrode distance of 1.5 cm. The Artificial Neural Network (ANN) technique was used to model the experimental data of the current density. The feed-forward neural network model was optimized by using the Levenberg-Marquardt algorithms. A comparison between the predicted and experimental data gave high correlation coefficients (0.99977 and 1) with the minimum MSE value (1.55.10-7 and 1.31.10-5) respectively for Al and Fe electrodes.

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[1] Rawat D., Mishra V., Sharma R.S., Detoxification of Azo Dyes in the Context of Environmental Processes, Chemosphere, 155: 591–605  (2016).
[2] Sanjay K., Sharma, ‎Rashmi Sanghi., Wastewater Reuse and Management, (2013).
[3] Boukerroui A., Meziti Ch., Reuse of Solid Waste in Adsorption of the Textile Dye Conference Title: Eight International Conference on Material Sciences (CSM8), Physics Procedia, 55: 173-178 (2014).
[4] Kamranifar M., Naghizadeh A., Montmorillonite Nanoparticles in Removal of Textile Dyes from Aqueous Solutions: Study of Kinetics and Thermodynamics, Iran. J. Chem. Chem. Eng. (IJCCE), 36(6): 127-137 (2017).
[5] Guimarães J.R., Maniero M.G., Nogueira de Araújo R., A Comparative Study on the Degradation of RB-19 Dye in An Aqueous Medium by Advanced Oxidation Processes, J. Environ. Manage, 110: 33-39 (2012).
[6] Nandi B.K., Patel S., Effects of Operational Parameters on the Removal of Brilliant Green Dye from Aqueous Solutions by Electrocoagulation, Arabian Journal of Chemistry, 10: 2961-2968 (2017).
[7] De Carvalho H.P., Huang J., Zhao M., Liu G., Dong L., Xingjuan Liu., Improvement of Methylene Blue Removal by Electrocoagulation/banana Peel Adsorption Coupling in a Batch System, Alexandria Engineering Journal, 54: 777–786 (2015).
[8] Kon H., Kusumoto R., Removal of Anionic Dyes in Aqueous Solution by Flocculation with Cellulose Ampholytes, Journal of Water Process Engineering, 7: 83–93 (2015).
[9] Avsar Y., Kurt U., Gonullu T., Comparison of Classical Chemical and Electrochemical Processes for Treating Rose Processing Wastewater, J. Hazard. Mater, 148: 340–345 (2007).
[10] Mollah M.Y.A., Schennach R., Parga J.R., Cocke D.L., Electrocoagulation (EC)—Science and Applications, J. Hazard. Mater, 84: 29-41 (2001).
[11] Ghosh D., Solanki H., Purkait M.K., Removal of Fe(II) from Tap Water by Electro Coagulation Technique, J. Hazard. Mater, 155: 135-143 (2008).
[12] Yahiaoui O., Aizel L., Lounici H., Drouiche N., Goosen M.F.A., Pauss A., Mameri N., Evaluating Removal of Metribuzin Pesticide from Contaminated Groundwater Using an Electrochemical Reactor Combined with Ultraviolet Oxidation, Desalination, 270: 84-89 (2011).
[13] Heidmann I., Calmano V., Removal of Zn (II), Cu (II), Ni (II), Ag (I) and Cr (VI) Present in Aqueous Solutions by Aluminium Electro Coagulation,  J. Hazard. Mater, 152(3): 934-941 (2008).
[14] Hakizimana J.N., Gourich B., Chafi M., Stiriba Y., Vial C., Drogui P., Naja J., Electrocoagulation Process in Water Treatment: A Review of Electrocoagulation Modeling Approaches, Desalination, 404:1–21 (2017).
[15] Tirado L., Gökkuş Ö., Brillas E., Sirés I., Treatment of Cheese Whey Wastewater by Combined Electrochemical Processes, J. Appl. Electrochem., (2018). [In Press].
[16] Secula M.S., Cagnon B., Ferreira d’Oliveira T., Cedarville O., Fauduet H., Removal of Acid Dye from Aqueous Solutions by Electrocoagulation/GAC Adsorption Coupling: Kinetics and Electrical Operating Costs, Journal of the Taiwan Institute of Chemical Engineers, 43:767–775 (2012).
[17] Feng J.W., Sun  Y.B., Zheng  Z., Zhan, J.B., Li  S., Tian Y.C., Treatment of Tannery Wastewater by Electrocoagulation, J. Environ. Sci, 19: 1409-1415 (2007).
[18] Ahmadu  F.R., Pendashteh  A., Abdullah  L.C., Biak  D.R.A., Madaeni  S.S., Abidin  Z.Z., Review of Technologies for Oil and Gas Produced Water Treatment, J. Hazard Mater, 170: 530-551 (2009).
[19] Nagata Y., Chu K.H., Optimization of a Fermentation Medium Using Neural Networks and Genetic Algorithms, Biotechnology Letters, 25: 1837–1842 (2003).
[20] Daneshvar N., Ashassi-Sorkhabi H., Tizpar A., Decolorization of Orange II by Electrocoagulation Method, Sep. Purif. Technol, 31: 153–162 (2003).
[21] Khandegar V., Saroha  AK., Electrochemical Treatment of Textile Effluent Containing Acid Red 131 Dye, Journal of Hazardous, Toxic,  (2013).
[22] Shokri Aref., Application of Electrocoagulation Process for the Removal of Acid Orange 5 in Synthetic Wastewater, Iran. J. Chem. Chem. Eng (IJCCE), 38 (2): 113-119 (2019).
[23] Liu F., Zhang Z., Wang Z., Li X., Dai X., Wang L., Wang X., Yuan Z., Zhang J., Chen M., Wang S., Experimental Study on Treatment of Tertiary Oil Recovery Wastewater by Electrocoagulation, Chem. Eng. Process, 144: (2019).
[24] Adhoum N., Monser L., Bellakhal N., Belgaied J.E., Treatment of Electroplating Wastewater Containing Cu2+, Zn2+ and Cr(VI) by Electrocoagulation, J. Hazard. Mater, 112(3): 207–2013 (2004).
[25] Varank G., Erkan H., Yazici S., Demir A., Engin G., Electrocoagulation of Tannery Wastewater Using Monopolar Electrodes: Process Optimization by Response Surface Methodology, Int. J. Environ. Res., 8(1):165–180 (2014).
[26] Mohajeri S., Hamidi A.A., Isa M.H., Zahed M.A., Landfill Leachate Treatment Through Electro-Fenton Oxidation, Pollution, 5(1):199–209 (2019).
[27] Elabbas S., Ouazzani N., Mandi L., Berrekhis F., Perdicakis M., Pontvianne S., M.-N. Pons F. Lapicque, J.-P. Leclerc, Treatment of Highly Concentrated Tannery Wastewater Using Electrocoagulation: Influence of the Quality of Aluminium Used for the Electrode, Journal of Hazardous Materials, 319: 69-77 (2016).
[28] Mouedhen G., Feki M., Wery M.D.P., Ayedi H.F., Behavior of Aluminum Electrodes in Electrocoagulation Process, J. Hazard. Mater., 150: 124-135 (2008).
[29] Karagozoğlu B., Malkoç R., The Investigation of the Removal of Reactive or- Ange 16 Dye from Textile Wastewater by Using Electrocoagulation Process, Cumhuriyet Sci. J., 38(3): 544-556 (2017).
[30] Daneshvar N., Ashassi-Sorkhabi H., Tizpar A., Decolorization of Orange II by Electrocoagulation Method, Sep. Purif. Technol., 31: 153–162 (2003).
[31] Khorram A.G., Fallah N., Treatment of Textile Dyeing Factory Wastewater by Electrocoagulation with Low Sludge Settling Time: Optimization of Operating Parameters by RSM, J. Environ. Chem. Eng., 78(6): 635-642 (2018).
[32] Delil A.D., Goren N., Investigation of Electrocoagulation and Electrooxidation Methods of Real Textile Wastewater Treatment, Eskişehir Technical Univ. J. of Sci. and Tech. A - Appl. Sci. and Eng., 20(1): 80-91 (2019).
[33] Modirshahla N., Behnajady M., Kooshaiian S., Investigation of the Effect of Different Electrode Connections on the Removal Efficiency of Tartrazine from Aqueous Solutions by Electrocoagulation, Dyes Pigm., 74: 249-257 (2007).
[34] Ayhan I., Engil S., Mahmut O., The Decolorization of C.I. Reactive Black 5 in Aqueous Solution by Electrocoagulation Using Sacrificial Iron Electrodes, Journal of Hazardous Materials, 161: 1369–1376 (2009).
[35] Duran A., Monteagudo J.M., Solar Photocatalytic Degradation of Reactive Blue 4 Using a Fresnel Lens, Water Research, 41: 690-698 (2007).
[36] Zahedi Abghari S., Imani A., Determination of Suitable Operating Conditions of Fluid Catalytic Cracking Process by Application of Artificial Neural Network and Firefly Algorithm, Iran. J. Chem. Chem. Eng. (IJCCE), 37(6): 157- 166 (2018).
[37] Tarjomannejad A., Prediction of the Liquid Vapor Pressure Using the Artificial Neural Network-Group Contribution Method, Iran. J. Chem. Chem. Eng. (IJCCE), 34(4): 97 - 111 (2015).